vmkping failure indicates there is a misconfiguration with the IP, VLAN, or MTU.
Resolution
Verify that the IP address configured on the vmkernel adapter is in the same subnet as the NFS target.
For example, if the network for your NFS target and vmkernel adapters is a /25 CIDR (subnet mask 255.255.255.128) you have IPs ###.###.###.1 to ###.###.###.128 as available IPs that will be able to communicate with each other over Layer 2. ###.###.###.5 and ###.###.###.200 would not be able to communicate with each other as they are not in the same IP subnet.
Verify that the VLAN configuration on the NFS vmkernel port group is correct.