Adding a cloud account in VCF Automation gives a red banner with the error message "The specified vCenter or NSX Manager is already associated with an existing region and cannot be reused. To use it in a VM Apps organization, ensure the vCenter or NSX Manager is not assigned to any region."
VCF Automation 9.0.0
This issue occurs if the vCenter endpoint is already in use by any All Apps organization in VCF Automation.
In VM Apps organization, use a vCenter endpoint that is not used by any All Apps organization or if the All Apps organization is not required, it can be deleted by following the documentation Delete a VCF Automation Organization.
When creating a new organization, consider the following key points: